Generation of millijoule few-cycle pulses at 5 μm by indirect spectral shaping of the idler in an optical parametric chirped pulse amplifier

Spectral pulse shaping in a high-intensity midwave-infrared (MWIR) optical parametric chirped pulse amplifier (OPCPA) operating at 1 kHz repetition rate is reported. We successfully apply a MWIR spatial light modulator (SLM) for the generation of ultrashort idler pulses at 5 μm wavelength. Only bulk optics and active phase control of the 3.5 μm signal pulses via the SLM are employed for generating compressed idler pulses with a duration of 80 fs. The 80-fs pulse duration corresponds to less than five optical cycles at the central wavelength of 5.0 μm. The pulse energy amounts to 1.0 mJ, which translates into a peak power of 10 GW. The generated pulse parameters represent record values for high-intensity MWIR OPCPAs

Double tungstate lasers: From bulk toward on-chip integrated waveguide devices

It has been recognized that the monoclinic double tungstates $KY{(WO_4)}_2$, $KGd{(WO_4)}_2$, and $KLu{(WO_4)}_2$ possess a high potential as rare-earth-ion-doped solid-state laser materials, partly due to the high absorption and emission cross sections of rare-earth ions when doped into these materials. Besides, their high refractive indexes make these materials potentially suitable for applications that require optical gain and high power in integrated optics, with rather high integration density. We review the recent advances in the field of bulk lasers in these materials and present our work toward the demonstration of waveguide lasers and their integration with other optical structures on a chip

Few-cycle 65-µJ pulses at 11.4 µm for ultrafast nonlinear longwave-infrared spectroscopy

Low-energy excitations can provide insight into the basic ultrafast nonequilibrium dynamics of condensed matter. High-energy femtosecond pulses in the long-wavelength infrared are required to induce such processes, and can be generated in an optical parametric chirped pulse amplification (OPCPA) system comprising three GaSe stages. A femtosecond Cr:ZnS laser serves as the front-end, providing the seed for the 2.0-µm pump and the 2.4-µm signal pulses without nonlinear conversion processes. The OPCPA system is pumped at 2.05 µm by a picosecond Ho:YLF regenerative amplifier at a 1-kHz repetition rate. The recompressed idler pulses at 11.4 µm have a duration of 185 fs and an unprecedented energy of 65 µJ, corresponding to a pump-to-idler conversion efficiency of 1.2%. Nonlinear transmission experiments in the range of the L2 infrared band of liquid water demonstrate the potential of the pulses for nonlinear vibrational spectroscopy of liquids and solids

Multi-millijoule, few-cycle 5 µm OPCPA at 1 kHz repetition rate

A table-top midwave-infrared optical parametric chirped pulse amplification (OPCPA) system generates few-cycle pulses with multi-10 GW peak power at a 1 kHz repetition rate. The all-optically synchronized system utilizes ZnGeP2 nonlinear crystals and a highly stable 2 µm picosecond pump laser based on Ho:YLiF4. An excellent energy extraction is achieved by reusing the pump pulse after the third parametric power amplification stage, resulting in 3.4 mJ idler pulses at a center wavelength of 4.9 µm. Pulses as short as 89.4 fs are achieved, close to only five optical cycles. Taking into account the pulse energy, a record high peak power of 33 GW for high-energy mid-IR OPCPAs beyond 4 µm wavelength is demonstrated. © 2020 OSA - The Optical Society. All rights reserved

Femtosecond-laser-written hexagonal cladding waveguide in Tm:KLu(WO_4)_2: µ-Raman study and laser operation

We report on the fabrication, µ-Raman characterization, and continuous-wave laser operation of a channel waveguide with a hexagonal optical-lattice-like cladding fabricated in monoclinic Tm:KLu(WO4)2 crystal by femtosecond direct laser writing. µ-Raman spectroscopy indicates preservation of the crystalline quality in the core region and an anisotropic residual stress field. When pumped by a Ti:Sapphire laser at 802 nm, the Tm:KLu(WO4)2 buried channel waveguide laser generated 136 mW at 1843.7 nm with a slope efficiency of 34.2% and a threshold as low as 21 mW, which are the record characteristics for femtosecond-laser-written Tm crystalline waveguide lasers. The variation of the output coupling resulted in discrete wavelength tuning of the laser emission from 1785 to 1862 nm. The propagation losses in the waveguide are ~1.2 ± 0.3 dB/cm.E. K. acknowledges financial support from the Generalitat de Catalunya under grants 2016FI_B00844 and 2017FI_B100158. F.D. acknowledges additional support through the ICREA academia award 2010ICREA-02 for excellence in research. X. M. acknowledges support from the European Union’s Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement No 657630. A. R. acknowledges funding from the European Union’s Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie Individual Fellowship Grant Agreement No. 747055. P. L. acknowledges financial support from the Government of the Russian Federation (Grant 074-U01) through ITMO Post-Doctoral Fellowship scheme

Oriented zinc oxide nanorods: A novel saturable absorber for lasers in the near-infrared

Zinc oxide (ZnO) nanorods (NRs) oriented along the crystallographic [001] axis are grown by the hydrothermal method on glass substrates. The ZnO NRs exhibit a broadband (1–2 µm) near-IR absorption ascribed to the singly charged zinc vacancy VZn−1. The saturable absorption of the ZnO NRs is studied at ≈1 µm under picosecond excitation, revealing a low saturation intensity, ≈10 kW/cm2, and high fraction of the saturable losses. The ZnO NRs are applied as saturable absorbers in diode-pumped Yb (≈1.03 µm) and Tm (≈1.94 µm) lasers generating nanosecond pulses. The ZnO NRs grown on various optical surfaces are promising broadband saturable absorbers for nanosecond near-IR lasers in bulk and waveguide geometries

Efficient tunable laser operation of Tm:KGd(WO4)2 in the continuous-wave regime at room temperature

Tm:KGd(WO/sub 4/)/sub 2/ is studied as a three-level laser on the /sup 3/F/sub 4/ /spl rarr/ /sup 3/H/sub 6/ transition and a tunable source in the 2-/spl mu/m spectral range, operating at room temperature. An overall tunability extending from 1790 to 2042 nm is achieved with maximum output powers of 400 mW for an absorbed pump power of 1 W. Various doping levels, pump wavelengths and polarization configurations are compared and the advantages of the monoclinic double tungstates over other Tm-hosts are outlined

Graphene Q-switched Yb:KYW planar waveguide laser

A diode-pumped Yb:KYW planar waveguide laser, single-mode Q-switched by evanescent-field interaction with graphene, is demonstrated for the first time. Few-layer graphene grown by chemical vapor deposition is transferred onto the top of a guiding layer, which initiates stable Q-switched operation in a 2.4-cm-long waveguide laser operating near 1027 nm. Average output powers up to 34 mW and pulse durations as short as 349 ns are achieved. The measured output beam profile, clearly exhibiting a single mode, agrees well with the theoretically calculated mode intensity distribution inside the waveguide. As the pump power is increased, the repetition rate and pulse energy increase from 191 to 607 kHz and from 7.4 to 58.6 nJ, respectively, whereas the pulse duration decreases from 2.09 μs to 349 ns

Comparative spectroscopic and thermo-optic study of Tm: LiLnF4 (Ln = Y, Gd, and Lu) crystals for highly-efficient microchip lasers at ~2 μm

We report on a detailed comparative study of the spectroscopic and thermo-optic properties of tetragonal Tm:LiLnF4 (Ln = Y, Gd, and Lu) crystals indicating their suitability for highly-efficient microchip lasers diode-pumped at ~791 nm and operating at ~1.91 μm. An a-cut 8 at.% Tm:LiYF4 micro-laser generated 3.1 W of linearly polarized output at 1904 nm with a slope efficiency of η = 72% and a laser threshold of only 0.24 W. The internal loss for this crystal is as low as 0.0011 cm-1. For 8 at.% Tm:LiGdF4 and 12 at.% Tm:LiLuF4 lasers, the output power reached ~2 W and η was 65% and 52%, respectively. The thermal lens in all Tm:LiLnF4 crystals is weak, positive and low-astigmatic. The potential for the Tm:LiLnF4 lasers to operate beyond ~2 μm due to a vibronic coupling has been proved. The Tm:LiYF4 vibronic laser generated 375 mW at 2026-2044 nm with η = 31%. The Tm:LiLnF4 crystals are very promising for passively Q-switched microchip lasers